Optimization of the synthesis of salts [V10O28]6– for the preparation of [VO2(DMSO)4](CF3SO3) and its immobilization on polyethylene terephthalate for catalytic applications

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Дәйексөз келтіру

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Аннотация

Aspects of the synthesis and isolation of (Bu4N)3[H3V10O28] (I) and Na6[V10O28] · 18H2O (II) from one reaction mixture are considered. The procedure for the synthesis of compound I is optimized. The reaction of compound I and HSO3CF3 in dimethyl sulfoxide (DMSO) affords complex [VO2(DMSO)4](CF3SO3) (III). A possibility of using complex III for the preparation of catalytically active materials based on polyethylene terephthalate (PET) is shown.

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Авторлар туралы

P. Abramov

Nikolaev Institute of Inorganic Chemistry, Siberian Branch, Russian Academy of Sciences

Хат алмасуға жауапты Автор.
Email: abramov@niic.nsc.ru
Ресей, Novosibirsk

N. Kompan’kov

Nikolaev Institute of Inorganic Chemistry, Siberian Branch, Russian Academy of Sciences

Email: abramov@niic.nsc.ru
Ресей, Novosibirsk

V. Sulyaeva

Nikolaev Institute of Inorganic Chemistry, Siberian Branch, Russian Academy of Sciences

Email: abramov@niic.nsc.ru
Ресей, Novosibirsk

M. Sokolov

Nikolaev Institute of Inorganic Chemistry, Siberian Branch, Russian Academy of Sciences

Email: abramov@niic.nsc.ru
Ресей, Novosibirsk

Әдебиет тізімі

  1. Pope M.T. Heteropoly and Isopoly Oxometalates. Berlin: Springer-Verlag, 1983. https://www.springer.com/gp/book/9783662120064 (accessed September 21, 2017)
  2. Kozhevnikov I.V. // Polyoxometal. Mol. Sci. 2003. V. 98. P. 351.
  3. Kozhevnikov I.., Kloetstra K.., Sinnema A. et al. // J. Mol. Catal. A. 1996. V. 114. № 1–3. P. 287. https://doi.org/10.1016/S1381-1169(96)00328-7
  4. Johnson H.N., Kirkbright G.F., Whitehouse R.J. // Anal. Chem. 1973. V. 45. № 9. P. 1603. https://doi.org/10.1021/ac60331a032
  5. Dubovik D.B., Tikhomirova T.I., Ivanov A.V. et al. // J. Anal. Chem. 2003. V. 58. P. 802. https://doi.org/10.1023/A:1025672831189
  6. Negrin A. // Clin. Chem. 1969. V. 15. № 9. P. 829. https://doi.org/10.1093/clinchem/15.9.829
  7. Scott J.E. // J. Histochem. Cytochem. 1971. V. 19. № 11. P. 689. https://doi.org/10.1177/19.11.689
  8. Sternberg M.Z. // Biotechnol. Bioeng. 1970. V. 12. № 1. P. 1. https://doi.org/10.1002/bit.260120102
  9. Yamase T. // Mol. Eng. 1993. V. 3. № 1–3. P. 241. https://doi.org/10.1007/BF00999636
  10. Raza R., Matin A., Sarwar S. et al. // Dalton Trans. 2012. V. 41. № 47. P. 14329. https://doi.org/10.1039/c2dt31784b
  11. Moore F.W., Tsigdinos G.A. // J. Less Common Met. 1977. V. 54. № 1. P. 297. https://doi.org/10.1016/0022-5088(77)90151-5
  12. Tsigdinos G.A. // Top. Curr. Chem. 1978. p. 14. https://doi.org/10.1007/BFb0047026
  13. Miras H.N., Cooper G.J.T., Long D.-L. et al. // Science.. 2010. V. 327. № 5961. P. 72. https://doi.org/10.1126/science.1181735
  14. Christie L.G., Surman A.J., Scullion R.A. et al. // Angew. Chem. Int. Ed. 2016. V. 55. № 41. P. 12741. https://doi.org/10.1002/anie.201606005
  15. Müller A., Kögerler P., Dress A.W.M.W.M. // Coord. Chem. Rev. 2001. V. 222. № 1. P. 193. https://doi.org/10.1016/S0010-8545(01)00391-5
  16. Lian X.-K., Chen H.-B., Lin Y.-D. et al. // Coord. Chem. Rev. 2023. V. 497. P. 215440. https://doi.org/10.1016/j.ccr.2023.215440
  17. Lv W., Han S.-D., Li X.-Y. et al. // Coord. Chem. Rev. 2023. V. 495. P. 215376. https://doi.org/10.1016/j.ccr.2023.215376
  18. Granadeiro C.M., Julião D., Ribeiro S.O. et al. // Coord. Chem. Rev. 2023. V. 476. P. 214914. https://doi.org/10.1016/j.ccr.2022.214914
  19. Zhang H., Li A., Li K. et al. // Nature. 2023. V. 616. № 7957. P. 482. https://doi.org/10.1038/s41586-023-05840-z
  20. Nyman M., Deblonde G. // Nature. 2023. V. 616. № 7957. P. 438. https://doi.org/10.1038/d415860023001019-8
  21. Liu C., Zhang Z., Liu W. et al. // Green Energy Environ. 2017. V. 2. № 4. P. 436. https://doi.org/10.1016/j.gee.2016.12.003
  22. Cai X., Xu Q., Tu G. et al. // Front. Chem. 2019. V. 7:42.? https://doi.org/10.3389/fchem.2019.00042
  23. Song J., Luo Z., Britt D.K. et al. // J. Am. Chem. Soc. 2011. V. 133. № 42. P. 16839. https://doi.org/10.1021/ja203695h
  24. Monakhov K.Y., Bensch W., Kögerler P. // Chem. Soc. Rev. 2015. V. 44. № 23. https://doi.org/10.1039/C5CS00531K
  25. Wendt M., Warzok U., Näther C. et al. // Chem. Sci. 2016. V. 7. № 4. P. 2684. https://doi.org/10.1039/C5SC04571A
  26. Ma P., Hu F., Wang J. et al. // Coord. Chem. Rev. 2018. V. 378. P. 281. https://doi.org/10.1016/J.CCR.2018.02.010
  27. Aureliano M., Gumerova N.I., Sciortino G. et al. // Coord. Chem. Rev. 2021. V. 447. P. 214143. https://doi.org/10.1016/j.ccr.2021.214143
  28. Wang J., Liu X., Du Z. et al. // Dalton Trans. 2021. V. 50. № 23. P. 7871. https://doi.org/10.1039/D1DT00494H
  29. Li J., Zhang D., Chi Y. et al. // Polyoxometalates. 2022. V. 1. № 2. P. 9140012. https://doi.org/10.26599/POM.2022.9140012
  30. Anjass M., Lowe G.A., Streb C. // Angew. Chem. Int. Ed. 2021. V. 60. № 14. P. 7522. https://doi.org/10.1002/anie.202010577
  31. Fraqueza G., Aureliano M. // BiTaP MDPI. 2022, p. 8 https://doi.org/10.3390/BiTaP-12844
  32. Shuvaeva O. V., Zhdanov A.A., Romanova T.E. et al. // Dalton Trans. 2017. V. 46. № 11. P. 3541. https://doi.org/10.1039/C6DT04843A
  33. Volchek V. V., Kompankov N.B., Sokolov M.N. et al. // Molecules. 2022. V. 27. № 23. P. 8368. https://doi.org/10.3390/molecules27238368
  34. Sheldrick G.M. // Acta Crystallogr. A. 2015. V. 71. № 1. P. 3. https://doi.org/10.1107/S2053273314026370
  35. Sheldrick G.M. // Acta Crystallogr. C. 2015. V. 71. № 1. P. 3. https://doi.org/10.1107/S2053229614024218
  36. Hübschle C.B., Sheldrick G.M., Dittrich B. // J. Appl. Crystallogr. 2011. V. 44. № 6. P. 1281. https://doi.org/10.1107/S0021889811043202
  37. Klemperer W.G. // Inorg. Synth. 1990. p. 74. https://doi.org/10.1002/9780470132586.ch15
  38. Domaille P.J. // J. Am. Chem. Soc. 1984. V. 106. № 25. P. 7677. https://doi.org/10.1021/ja00337a004
  39. Durif A., Averbuch-Pouchot M.T., Guitel J.C. // Acta Crystallogr. B. 1980. V. 36. № 3. P. 680. https://doi.org/10.1107/S0567740880004116
  40. Bošnjaković-Pavlović N., Prévost J., Spasojević-de Biré A. // Cryst. Growth Des. 2011. V. 11. № 9. P. 3778. https://doi.org/10.1021/cg200236d
  41. Krakowiak J., Lundberg D., Persson I. // Inorg. Chem. 2012. V. 51. № 18. P. 9598. https://doi.org/10.1021/ic300202f
  42. Guselnikova O., Svanda J., Postnikov P. et al. // Adv. Mater. Interfaces. 2017. V. 4. № 5. https://doi.org/10.1002/admi.201600886
  43. Guselnikova O., Elashnikov R., Postnikov P. et al. // ACS Appl. Mater. Interfaces. 2018. V. 10. № 43. P. 37461. https://doi.org/10.1021/acsami.8b06840
  44. Guselnikova O., Barras A., Addad A. et al. // Sep. Purif. Technol. 2020. V. 240. P. 116627. https://doi.org/10.1016/j.seppur.2020.116627
  45. Guselnikova O., Semyonov O., Kirgina M. et al. // J. Environ. Chem. Eng. 2022. V. 10. № 2. P. 107105. https://doi.org/10.1016/j.jece.2021.107105
  46. Semyonov O., Chaemchuen S., Ivanov A. et al. // Appl. Mater. Today. 2021. V. 22. P. 100910. https://doi.org/10.1016/j.apmt.2020.100910
  47. Kogolev D., Semyonov O., Metalnikova N. et al. // J. Mater. Chem. A. 2023. V. 11. № 3. P. 1108. https://doi.org/10.1039/D2TA08127J
  48. Guselnikova O., Semyonov O., Sviridova E. et al. // Chem. Soc. Rev. 2023. V. 52. № 14. P. 4755. https://doi.org/10.1039/D2CS00689H
  49. Licini G., Conte V., Coletti A. et al. // Coord. Chem. Rev. 2011. V. 255. № 19–20. P. 2345. https://doi.org/10.1016/j.ccr.2011.05.004
  50. Langeslay R.R., Kaphan D.M., Marshall C.L. et al. // Chem. Rev. 2019. V. 119. № 4. P. 2128. https://doi.org/10.1021/acs.chemrev.8b00245
  51. Maksimchuk N. V., Kholdeeva O.A., Kovalenko K.A. et al. // Isr. J. Chem. 2011. V. 51. № 2. P. 281. https://doi.org/10.1002/ijch.201000082
  52. Evtushok V.Y., Suboch A.N., Podyacheva O.Y. et al. // ACS Catal. 2018. V. 8. № 2. P. 1297. https://doi.org/10.1021/acscatal.7b03933
  53. Rodikova Y.A., Zhizhina E.G., Pai Z.P. // Appl. Catal. A. 2018. V. 549. P. 216. https://doi.org/10.1016/j.apcata.2017.09.022
  54. Palion-Gazda J., Luz A., Raposo L.R. et al. // Molecules. 2021. V. 26. № 21. P. 6364. https://doi.org/10.3390/molecules26216364
  55. Zhao L., Yang P., Shi S. et al. // ACS Catal. 2022. V. 12. № 24. P. 15249. https://doi.org/10.1021/acscatal.2c04601
  56. Kikukawa Y., Sakamoto Y., Hirasawa H. et al. // Catal. Sci. Technol. 2022. V. 12. № 8. P. 2438. https://doi.org/10.1039/D1CY02103F
  57. Fomenko I.S., Gushchin A.L., Abramov P.A. et al. // Catalysts. 2019. V. 9. № 3.

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2. Fig. 1. Comparison of experimental XRD data (298 K) and calculated data obtained from PCA data (150 K) for complex I.

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3. Fig. 2. Comparison of experimental XRD data (298 K) and calculated data obtained from PCA data (150 K) for complex III.

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4. Fig. 3. Structure of the [V10O28]6- anion (a) and the [VO2(DMSO)4]+ cation (b). Spherical rod models, the hydrogen atoms of the methyl groups are not shown for clarity.

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5. Fig. 4. 51V NMR spectra of solutions of III (298 K) in (CD3)2SO (a), (CD3)2CO (b), D2O (c). Spectrum of complex I in CD3CN (d).

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6. Fig. 5. SEM image of the sample (a), EDX mapping of vanadium, oxygen and carbon and their joint image (b) and energy dispersive spectrum (c).

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